The 1967 Spider-Man series is a bit deceptive, as it is really two different shows rolled into one.
The first season was created by some Canadian animation company called Grantray-Lawrence Animation, and it's generally the extremely campy version of this show that most are familiar with. Characters were very one dimensional, Jamison was hilariously awesome. Plots were just silly.
Season 2 and 3 on the other hand were directed by Ralph Bakshi's animation company in New York, and was a reboot of the series. Season 2 and 3 completely changed the character personalities of all the main cast. It tried to make them more fleshed out and a bit darker in tone. Jamison in season 2 and 3 was a lot more subdued than his wacky counterpart in the first season, and these seasons focused more on Peter Parker's character. But sadly the budget was smaller compared to the first season, which forced the animators to recycle frames of animation from season 1. But the original art and animation that was produced for season two had much better framing, nicer painted backgrounds and was a little more stylish than season one. But there was also this really bad clashing of styles between the season 1 and season 2 animation. By season 3 though the show got really psychedelic and weird as they were recycling animation from other shows that weren't Spider-Man related.
I kinda did like season two and three of the 1960's show, for what it was. If only Bakshi had a bigger budget, his version could've been really awesome.
Also, on the list. I really enjoyed the 1994 Spider-Man a lot when I was a kid. I really liked the crossovers it had with the X-men series. The Spectacular Spider-Man was great too, but those designs always felt a tad bit off with me. I dunno.
cartoon = animated series? if so then hell fucking no.
This is the GOAT.
Nothing will ever beat this series, NOTHING.
This still sits as my number 1 comic book adaption. Though I always kinda liked the HBO Spawn animated series as well, even though it had some dodgy animation. The MaXX was another one, it was short but I really loved the art in that one.