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I'm mostly looking for things that work especially well on Wii U or are exclusive to it. I have already played or had an opportunity to buy most of your recommendations on PC. I would include VC, but I guess that library is so big that it's hard to narrow it down. I'm basically looking for experiences I wouldn't get on my PC.

Wii U VC is very limited. Note that you cannot use your eShop funds on the Wii Shop Channel in Wii Mode where all the old Wii VC and WiiWare stuff lives.