So i'm reading the optimal sharpness setting for older CRTs is 0?
Yep. adding sharpness may be good for live action films, but it's definitely not for videogames or animation. And even for film I have my doubts. Turn it down to zero.
Some thoughts about it
http://www.lockergnome.com/media/2011/08/22/what-is-video-sharpness-on-a-television/
The option to sharpen the image produced by an CRTs video circuit has
basically nothing to do with sharpening the image as we know it today. The
sort of sharpening seen in CRTs is a post-emphasis filter to counter the long
roll-off and dumping of the higher frequencies produced by the video amplifier
circuits and their RC couplings. Pi-filters and similar ones are used to
emphasize the higher video frequencies again and to produce a faster roll-off
of the filter curve beyond the highest video frequency of the CRT to
eliminate much higher (left over) frequencies which could turn your amplifier
into an oscillator. However, it was found out that using those filters could
make the picture look more hires and were as such abused for marketing, i.e.
adjusted to produce a little plastic (as it is known) by pushing the higher
video frequencies more than necessary, whereas their original intent was just
to counter the deficiencies of the video amplifiers.
One only needs to adjust the sharpening feature up to the point where the
edges in the image start to get sort of an outline. Anything beyond just
serves the artist.